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By Charles E. Taylor, Jonathan T. Kwan

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Phys. Rev. , 2002, 88, 206105. ; Pusztai, T. J. Cryst. , 2002, 237–239, 1813. Davidchack, R. ; Laird, B. B. J. Chem. , 1998, 108, 9452. Oxtoby, D. W. Annu. Rev. Mater. , 2002, 32, 39. ; Conti, M; Kvamme, B. J. Chem. Phys. 2003, 119, 10376. 16. ; Jones, J. Ann. Phys. ), 1995, 237, 66. 17. Shen, Y. ; Oxtoby, D. W. J. Chem. , 1996, 105, 6517. 18 L. Gránásy et al. 18. Wang, S. ; Sekerka, R. ; Wheeler, A. ; Murray, B. ; Coriell, S. ; Braun, R. ; McFadden, G. B. Physica D, 1993,69, 189. 19. Cahn, J. ; Hilliard, J.

But stable structure-II large cavity can be built around two small guest molecules. We see that the explanation of this effect is the same as in previous case of structure II formation by extremely small molecules, and similar mechanism of structure I – structure II transformation of nuclei works. Thus, the role of multiple filling of cages in kinetic mechanisms of hydrate formation is decisive. It is interesting to investigate also the role of multiple filling in thermodynamic properties of hydrates.

Braun, R. ; McFadden, G. B. Physica D, 1993,69, 189. 19. Cahn, J. ; Hilliard, J. E. J. Chem. Phys, 1958, 28, 258; 1959, 31, 688. 20. Kelton, K. F. , 1991,45, 75. 21. Kelton, K. ; Greer, A. L. Phys. Rev. B, 1988, 38, 10089. 22. ; Warren, J. ; Douglas, J. ; Ferreiro, V. , 2003, 2, 92. 23. ,Warren, J. ; Carter, W. C. Physica D, 1998, 119, 415. 24. Warren, J. ; Douglas, J. F. Proc. TMS Ann. Meeting, San Francisco, 2004, accepted for publication. 25. ; Tanaka, H. J. Phys. , 1995, 99, 7114. 26. Kvamme, B.

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